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Free, publicly-accessible full text available April 1, 2026
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Ferroelectric nematic liquid crystals are fluids exhibiting spontaneous electric polarization, which is coupled to their long range orientational order. Due to their inherent property of making bound and surface charges, the free surface of ferroelectric nematics becomes unstable in electric fields. Here we show that ferroelectric liquid bridges between two electrode plates undergo distinct interfacial instabilities. In a specific range of frequency and voltage, the ferroelectric fluid bridges move as active interacting particles resembling living organisms like swarming insects, microbes or microrobots. The motion is accompanied by sound emission, as a consequence of piezoelectricity and electrostriction. Statistical analysis of the active particles reveals that the movement can be controlled by the applied voltage, which implies the possible application of the system in new types of microfluidic devices.more » « less
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Abstract Studies of sessile droplets and fluid bridges of a ferroelectric nematic liquid crystal in externally applied electric fields are presented. It is found that above a threshold, the interface of the fluid with air undergoes a fingering instability or ramification, resembling to Rayleigh-type instability observed in charged droplets in electric fields or circular drop-type instabilities observed in ferromagnetic liquids in magnetic field. The frequency dependence of the threshold voltage was determined in various geometries. The nematic director and ferroelectric polarization direction was found to point along the tip of the fingers that appear to repel each other, indicating that the ferroelectric polarization is essentially parallel to the director. The results are interpreted in connection to the Rayleigh and circular drop-type instabilities.more » « less
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Abstract Freestanding slender fluid filaments of room‐temperature ferroelectric nematic liquid crystals are described. They are stabilized either by internal electric fields of bound charges formed due to polarization splay or by external voltage applied between suspending wires. The phenomenon is similar to those observed in dielectric fluids, such as deionized water, except that in ferroelectric nematic materials the voltages required are three orders of magnitudes smaller and the aspect ratio is much higher. The observed ferroelectric fluid threads are not only unique and novel but also offer measurements of basic physical quantities, such as the ferroelectric polarization and viscosity. Ferroelectric nematic fluid threads may have practical applications in nano‐fluidic micron‐size logic devices, switches, and relays.more » « less
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Abstract The first demonstration of converse piezoelectricity in 3D fluids is presented by measuring a linear electromechanical effect in ferroelectric nematic liquid crystals. The observed piezoelectric coupling constant below 6 kHz electric field is larger than 1 nC/N, comparable to, or better than, values for the strongest solid piezoelectric materials. Symmetry considerations indicate that the alignment of the ferroelectric nematic liquid crystal in the experimental study is not optimized, so the observed signal is likely only a fraction of the theoretically achievable signal. Understanding the electromechanical response of ferroelectric nematics will enable mechanical energy harvesting and open up a new avenue for developing fluid actuators, micro positioners, and electrically tunable optical lenses.more » « less
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